Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams

R. Mateus; N. Catarino; M. Dias; L. C. Alves; O. Romanenko; Z. Siketić; I. Bogdanović Radović; A. Hakola; E. Grigore; E. Alves

doi:10.1016/j.nimb.2023.02.028

Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams

R. Mateus (Corresponding Author), N. Catarino, M. Dias, L. C. Alves, O. Romanenko, Z. Siketić, I. Bogdanović Radović, A. Hakola, E. Grigore, E. Alves,

BA4506 Fusion energy and decommissioning

Research output: Contribution to journal › Article › Scientific › peer-review

Abstract

Different studies reveal the behaviour of Ta alloying to decrease deuterium retention in tungsten bulk materials aiming to be used for nuclear fusion applications. In this work, W and W-5 %Ta coatings were produced via magnetron sputtering techniques. The elemental composition of the samples and the spread of Ta in the W lattice was confirmed by GDOES, PIXE and by μ-PIXE, respectively. Sets of W and W-Ta coatings were simultaneously irradiated with a single ²H₂⁺ or with sequential ⁴He⁺/²H₂⁺ ion beam implantations using incident energies of 30 keV and ion fluences of 5 × 10¹⁷ ion/cm². The irradiated samples were analysed by NRA/RBS and by ToF-ERDA to quantify the retained deuterium and helium amounts. The results reveal significantly lower contents of both isotopes in W-Ta.

Original language	English
Pages (from-to)	41-46
Number of pages	6
Journal	Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms
Volume	538
DOIs	https://doi.org/10.1016/j.nimb.2023.02.028
Publication status	Published - May 2023
MoE publication type	A1 Journal article-refereed

Keywords

Deuterium
Helium
Retention
W-Ta coatings

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Mateus, R., Catarino, N., Dias, M., Alves, L. C., Romanenko, O., Siketić, Z., Radović, I. B., Hakola, A., Grigore, E., Alves, E. (2023). Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams. Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms, 538, 41-46. https://doi.org/10.1016/j.nimb.2023.02.028

@article{1a57cde75d944b9fb07ced3b1157eb2f,

title = "Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams",

abstract = "Different studies reveal the behaviour of Ta alloying to decrease deuterium retention in tungsten bulk materials aiming to be used for nuclear fusion applications. In this work, W and W-5 %Ta coatings were produced via magnetron sputtering techniques. The elemental composition of the samples and the spread of Ta in the W lattice was confirmed by GDOES, PIXE and by μ-PIXE, respectively. Sets of W and W-Ta coatings were simultaneously irradiated with a single 2H2+ or with sequential 4He+/2H2+ ion beam implantations using incident energies of 30 keV and ion fluences of 5 × 1017 ion/cm2. The irradiated samples were analysed by NRA/RBS and by ToF-ERDA to quantify the retained deuterium and helium amounts. The results reveal significantly lower contents of both isotopes in W-Ta.",

keywords = "Deuterium, Helium, Retention, W-Ta coatings",

author = "R. Mateus and N. Catarino and M. Dias and Alves, {L. C.} and O. Romanenko and Z. Siketi{\'c} and Radovi{\'c}, {I. Bogdanovi{\'c}} and A. Hakola and E. Grigore and E. Alves",

note = "Funding Information: This work has been carried out within the framework of the EUROfusion Consortium, funded by the European Union via the Euratom Research and Training Programme (Grant Agreement No 101052200 - EUROfusion). Views and opinions expressed are however those of the author(s) only and do not necessarily reflect those of the European Union or the European Commission. Neither the European Union nor the European Commission can be held responsible for them. Work performed under EUROfusion WP PFC. The research leading to this result has been partially supported by Funda{\c c}{\~a}o para a Ci{\^e}ncia e a Tecnologia, Portugal, through projects UID/50010/2020 and PTDC/FIS-PLA/31629/2017, by the OP VVV project CZ.02.2.69/0.0/0.0/18_053/0017163 of the Czech Academy of Sciences and by the RADIATE project under the Grant Agreement 824096 from the EU Research and Innovation programme HORIZON 2020. Publisher Copyright: {\textcopyright} 2023",

year = "2023",

month = may,

doi = "10.1016/j.nimb.2023.02.028",

language = "English",

volume = "538",

pages = "41--46",

journal = "Nuclear Instruments and Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms",

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Mateus, R, Catarino, N, Dias, M, Alves, LC, Romanenko, O, Siketić, Z, Radović, IB, Hakola, A, Grigore, E, Alves, E 2023, 'Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams', Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms, vol. 538, pp. 41-46. https://doi.org/10.1016/j.nimb.2023.02.028

Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams. / Mateus, R. (Corresponding Author); Catarino, N.; Dias, M. et al.

In: Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms, Vol. 538, 05.2023, p. 41-46.

Research output: Contribution to journal › Article › Scientific › peer-review

TY - JOUR

T1 - Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams

AU - Mateus, R.

AU - Catarino, N.

AU - Dias, M.

AU - Alves, L. C.

AU - Romanenko, O.

AU - Siketić, Z.

AU - Radović, I. Bogdanović

AU - Hakola, A.

AU - Grigore, E.

AU - Alves, E.

N1 - Funding Information: This work has been carried out within the framework of the EUROfusion Consortium, funded by the European Union via the Euratom Research and Training Programme (Grant Agreement No 101052200 - EUROfusion). Views and opinions expressed are however those of the author(s) only and do not necessarily reflect those of the European Union or the European Commission. Neither the European Union nor the European Commission can be held responsible for them. Work performed under EUROfusion WP PFC. The research leading to this result has been partially supported by Fundação para a Ciência e a Tecnologia, Portugal, through projects UID/50010/2020 and PTDC/FIS-PLA/31629/2017, by the OP VVV project CZ.02.2.69/0.0/0.0/18_053/0017163 of the Czech Academy of Sciences and by the RADIATE project under the Grant Agreement 824096 from the EU Research and Innovation programme HORIZON 2020. Publisher Copyright: © 2023

PY - 2023/5

Y1 - 2023/5

N2 - Different studies reveal the behaviour of Ta alloying to decrease deuterium retention in tungsten bulk materials aiming to be used for nuclear fusion applications. In this work, W and W-5 %Ta coatings were produced via magnetron sputtering techniques. The elemental composition of the samples and the spread of Ta in the W lattice was confirmed by GDOES, PIXE and by μ-PIXE, respectively. Sets of W and W-Ta coatings were simultaneously irradiated with a single 2H2+ or with sequential 4He+/2H2+ ion beam implantations using incident energies of 30 keV and ion fluences of 5 × 1017 ion/cm2. The irradiated samples were analysed by NRA/RBS and by ToF-ERDA to quantify the retained deuterium and helium amounts. The results reveal significantly lower contents of both isotopes in W-Ta.

AB - Different studies reveal the behaviour of Ta alloying to decrease deuterium retention in tungsten bulk materials aiming to be used for nuclear fusion applications. In this work, W and W-5 %Ta coatings were produced via magnetron sputtering techniques. The elemental composition of the samples and the spread of Ta in the W lattice was confirmed by GDOES, PIXE and by μ-PIXE, respectively. Sets of W and W-Ta coatings were simultaneously irradiated with a single 2H2+ or with sequential 4He+/2H2+ ion beam implantations using incident energies of 30 keV and ion fluences of 5 × 1017 ion/cm2. The irradiated samples were analysed by NRA/RBS and by ToF-ERDA to quantify the retained deuterium and helium amounts. The results reveal significantly lower contents of both isotopes in W-Ta.

KW - Deuterium

KW - Helium

KW - Retention

KW - W-Ta coatings

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U2 - 10.1016/j.nimb.2023.02.028

DO - 10.1016/j.nimb.2023.02.028

M3 - Article

AN - SCOPUS:85149361942

SN - 0168-583X

VL - 538

SP - 41

EP - 46

JO - Nuclear Instruments and Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms

JF - Nuclear Instruments and Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms

ER -

Deuterium and helium retention in W and W-Ta coatings irradiated with energetic ion beams

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Keywords

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