Abstract
Solid oxide fuel cells (SOFC) can utilize various fuels,
such as natural gas, hydrogen and biogas, but often, it
is sensible to use a pre-reformer that converts the fuel
into a hydrogen-rich gas stream. Relevant testing
conditions, including the fuel to be used in SOFC
systems, are important because cell performance depends
on test conditions, such as fuel composition. Still, a
majority of the reported single-cell and short stack
tests are performed with pure hydrogen or synthetic
reformate mixed from gas bottles. In this article, the
development of a fuel feeder used to pre-reform natural
gas for a single cell SOFC test station is presented. To
mimic SOFC system conditions, natural gas is taken from
the grid, desulfurized with commercial sulfur sorbent and
reformed with a commercial precious metal catalyst. The
fuel feeder is designed to be a versatile and efficient
research tool, capable to be used in a wide temperature
and gas flow range and with different reforming
techniques, such as steam reforming, catalytic partial
oxidation and simulated anode off-gas recycling. The
construction, operation and characterization of the fuel
feeder as well as methods of avoiding carbon formation
are discussed. The performance is evaluated by comparing
measured outlet temperatures and compositions against
equilibrium values. All measured gas compositions matched
closely with the calculated equilibrium values, and the
identified deviations were small and to no harm in
practical use. The operator can control the product gas
composition by setting the fuel feeder heater to the
temperature corresponding to the targeted composition.
Results show that the fuel feeder design can be used as
such for single-cell testing or scaled to fit larger
stack test stations.
Original language | English |
---|---|
Pages (from-to) | 2031-2041 |
Journal | International Journal of Energy Research |
Volume | 39 |
Issue number | 15 |
DOIs | |
Publication status | Published - 2015 |
MoE publication type | A1 Journal article-refereed |
Keywords
- solid oxide fuel cell
- precious metal catalyst
- natural gas reforming
- single cell testing
- realistic test conditions