Effect of hydrogen on electrochemical behavior of additively manufactured 316L in pressurized water reactor primary water

Martin Bojinov; Timo Saario; Yanling Ge; Litao Chang; Zaiqing Que

doi:10.1016/j.corsci.2023.111557

Effect of hydrogen on electrochemical behavior of additively manufactured 316L in pressurized water reactor primary water

Martin Bojinov
, Timo Saario
, Yanling Ge
, Litao Chang
, Zaiqing Que^*

^*Corresponding author for this work

BA4509 Advanced materials for nuclear energy

University of Chemical Technology and Metallurgy
Shanghai Institute of Applied Physics (SINAP-CAS)

Research output: Contribution to journal › Article › Scientific › peer-review

6 Citations (Scopus)

288 Downloads (Pure)

Abstract

The electrochemical behavior of laser powder bed fusion (LPBF) 316 L stainless steel subject to different heat-treatments (solution annealing and hot isostatic pressing) is compared to nuclear-grade wrought 316 L in pressurized water reactor primary water at 288 °C (with and without dissolved hydrogen) using current-time transients, cyclic voltammetry and electrochemical impedance spectroscopy (EIS). Analysis of spectra by the Mixed-Conduction Model revealed slower corrosion rates of LPBF 316 L than wrought 316 L, the effect being more pronounced in the presence of dissolved hydrogen. The characteristics of the barrier layer and the oxide film/coolant interface were irreversibly altered upon removal of dissolved hydrogen.

Original language	English
Article number	111557
Journal	Corrosion Science
Volume	224
DOIs	https://doi.org/10.1016/j.corsci.2023.111557
Publication status	Published - Nov 2023
MoE publication type	A1 Journal article-refereed

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 9 Industry, Innovation, and Infrastructure

Keywords

Additive manufacturing
Corrosion
Dissolved hydrogen
High-temperature water
Laser powder bed fusion
Stainless steel

Access to Document

10.1016/j.corsci.2023.111557Licence: CC BY

j.corsci.2023.111557Final published version, 25.3 MBLicence: CC BY

Cite this

@article{fe71d30731c04ec0a8fad442d6caedcd,

title = "Effect of hydrogen on electrochemical behavior of additively manufactured 316L in pressurized water reactor primary water",

abstract = "The electrochemical behavior of laser powder bed fusion (LPBF) 316 L stainless steel subject to different heat-treatments (solution annealing and hot isostatic pressing) is compared to nuclear-grade wrought 316 L in pressurized water reactor primary water at 288 °C (with and without dissolved hydrogen) using current-time transients, cyclic voltammetry and electrochemical impedance spectroscopy (EIS). Analysis of spectra by the Mixed-Conduction Model revealed slower corrosion rates of LPBF 316 L than wrought 316 L, the effect being more pronounced in the presence of dissolved hydrogen. The characteristics of the barrier layer and the oxide film/coolant interface were irreversibly altered upon removal of dissolved hydrogen.",

keywords = "Additive manufacturing, Corrosion, Dissolved hydrogen, High-temperature water, Laser powder bed fusion, Stainless steel",

author = "Martin Bojinov and Timo Saario and Yanling Ge and Litao Chang and Zaiqing Que",

note = "The work is funded by VTT Substance Node Excellence Canva (GG\_PIETU\_Node), EU Horizon 2020 project MEACTOS (EURATOM research and training program 2014-2018, grant agreement no. 755151), Chinese Academy of Sciences (No. E051011031) and Innovation Funding of Shanghai Jiading District (No. E339031031).",

year = "2023",

month = nov,

doi = "10.1016/j.corsci.2023.111557",

language = "English",

volume = "224",

journal = "Corrosion Science",

issn = "0010-938X",

publisher = "Elsevier",

}

TY - JOUR

T1 - Effect of hydrogen on electrochemical behavior of additively manufactured 316L in pressurized water reactor primary water

AU - Bojinov, Martin

AU - Saario, Timo

AU - Ge, Yanling

AU - Chang, Litao

AU - Que, Zaiqing

N1 - The work is funded by VTT Substance Node Excellence Canva (GG_PIETU_Node), EU Horizon 2020 project MEACTOS (EURATOM research and training program 2014-2018, grant agreement no. 755151), Chinese Academy of Sciences (No. E051011031) and Innovation Funding of Shanghai Jiading District (No. E339031031).

PY - 2023/11

Y1 - 2023/11

N2 - The electrochemical behavior of laser powder bed fusion (LPBF) 316 L stainless steel subject to different heat-treatments (solution annealing and hot isostatic pressing) is compared to nuclear-grade wrought 316 L in pressurized water reactor primary water at 288 °C (with and without dissolved hydrogen) using current-time transients, cyclic voltammetry and electrochemical impedance spectroscopy (EIS). Analysis of spectra by the Mixed-Conduction Model revealed slower corrosion rates of LPBF 316 L than wrought 316 L, the effect being more pronounced in the presence of dissolved hydrogen. The characteristics of the barrier layer and the oxide film/coolant interface were irreversibly altered upon removal of dissolved hydrogen.

AB - The electrochemical behavior of laser powder bed fusion (LPBF) 316 L stainless steel subject to different heat-treatments (solution annealing and hot isostatic pressing) is compared to nuclear-grade wrought 316 L in pressurized water reactor primary water at 288 °C (with and without dissolved hydrogen) using current-time transients, cyclic voltammetry and electrochemical impedance spectroscopy (EIS). Analysis of spectra by the Mixed-Conduction Model revealed slower corrosion rates of LPBF 316 L than wrought 316 L, the effect being more pronounced in the presence of dissolved hydrogen. The characteristics of the barrier layer and the oxide film/coolant interface were irreversibly altered upon removal of dissolved hydrogen.

KW - Additive manufacturing

KW - Corrosion

KW - Dissolved hydrogen

KW - High-temperature water

KW - Laser powder bed fusion

KW - Stainless steel

UR - https://www.scopus.com/pages/publications/85172686094

U2 - 10.1016/j.corsci.2023.111557

DO - 10.1016/j.corsci.2023.111557

M3 - Article

SN - 0010-938X

VL - 224

JO - Corrosion Science

JF - Corrosion Science

M1 - 111557

ER -

Effect of hydrogen on electrochemical behavior of additively manufactured 316L in pressurized water reactor primary water

Abstract

UN SDGs

Keywords

Access to Document

Other files and links

Fingerprint

Cite this