Skip to main navigation Skip to search Skip to main content

Enhanced second-harmonic generation by single metal-insulator multilayered nanocavities with axial symmetry resonating in the near-infrared

  • Attilio Zilli*
  • , Tommi Isoniemi
  • , Marzia Iarossi
  • , Marco Finazzi
  • , Francesco De Angelis
  • , Michele Celebrano
  • , Nicolò Maccaferri*
  • *Corresponding author for this work
  • Polytechnic University of Milan
  • University of Sheffield
  • Istituto Italiano di Tecnologia (IIT)
  • University of Luxembourg

Research output: Chapter in Book/Report/Conference proceedingConference article in proceedingsScientificpeer-review

Abstract

We report efficient second-harmonic emission by single multilayer metal-dielectric nanocavities. Engineering the intrinsic interface-induced symmetry breaking by resonant optical absorption design, allows to achieve almost two orders of magnitude higher second-harmonic generation efficiency compared to gold nanostructures with the same geometry. We estimate a second-order nonlinear susceptibility of the order of 1 pm/V, which is comparable to widely used nonlinear crystals. We envision that our system, which combines the advantages of both plasmonic and dielectric materials, might enable the realization of composite nano-systems for an efficient multi-purpose manipulation of nonlinear optical processes at the nanoscale.

Original languageEnglish
Title of host publicationNonlinear Optics and Applications XII
EditorsMario Bertolotti, Anatoly V. Zayats, Alexei M. Zheltikov
PublisherInternational Society for Optics and Photonics SPIE
ISBN (Electronic)9781510643741
DOIs
Publication statusPublished - 2021
MoE publication typeA4 Article in a conference publication
EventNonlinear Optics and Applications XII 2021 - Virtual, Online, Czech Republic
Duration: 19 Apr 202123 Apr 2021

Publication series

SeriesProceedings of SPIE
Volume11770
ISSN0277-786X

Conference

ConferenceNonlinear Optics and Applications XII 2021
Country/TerritoryCzech Republic
CityVirtual, Online
Period19/04/2123/04/21

Keywords

  • Metal-dielectric
  • Metamaterials
  • Multilayers
  • Nanocavities
  • Nanophotonics
  • Nonlinear optics
  • Plasmonics
  • Second-harmonic generation

Fingerprint

Dive into the research topics of 'Enhanced second-harmonic generation by single metal-insulator multilayered nanocavities with axial symmetry resonating in the near-infrared'. Together they form a unique fingerprint.

Cite this