Interaction-time-averaged optical pumping in alkali-metal-atom Doppler spectroscopy

Thomas Lindvall, Ilkka Tittonen

Research output: Contribution to journalArticleScientificpeer-review

12 Citations (Scopus)

Abstract

We study the influence of optical pumping on Doppler-broadened alkali-metal-atom D line spectra by solving the time-dependent density matrix for an open two-level system. The time-dependent absorption is averaged over the distribution of interaction times obtained from the three-dimensional beam geometry and atomic velocity distribution and over the longitudinal velocity distribution. The optical pumping is significant at much lower intensities than saturation and depends strongly on the intensity, beam radius, vapor cell length, and spontaneous-decay branching ratio. The result is in agreement with our earlier steady-state solution for a wide range of parameters and predicts two interesting line-shape features.

Original languageEnglish
Article number032505
JournalPhysical Review A - Atomic, Molecular, and Optical Physics
Volume80
Issue number3
DOIs
Publication statusPublished - 9 Sep 2009
MoE publication typeA1 Journal article-refereed

Fingerprint

optical pumping
alkali metals
velocity distribution
spectroscopy
atoms
D lines
interactions
line spectra
line shape
vapors
saturation
radii
decay
geometry
cells

Cite this

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abstract = "We study the influence of optical pumping on Doppler-broadened alkali-metal-atom D line spectra by solving the time-dependent density matrix for an open two-level system. The time-dependent absorption is averaged over the distribution of interaction times obtained from the three-dimensional beam geometry and atomic velocity distribution and over the longitudinal velocity distribution. The optical pumping is significant at much lower intensities than saturation and depends strongly on the intensity, beam radius, vapor cell length, and spontaneous-decay branching ratio. The result is in agreement with our earlier steady-state solution for a wide range of parameters and predicts two interesting line-shape features.",
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Interaction-time-averaged optical pumping in alkali-metal-atom Doppler spectroscopy. / Lindvall, Thomas; Tittonen, Ilkka.

In: Physical Review A - Atomic, Molecular, and Optical Physics, Vol. 80, No. 3, 032505, 09.09.2009.

Research output: Contribution to journalArticleScientificpeer-review

TY - JOUR

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AU - Tittonen, Ilkka

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N2 - We study the influence of optical pumping on Doppler-broadened alkali-metal-atom D line spectra by solving the time-dependent density matrix for an open two-level system. The time-dependent absorption is averaged over the distribution of interaction times obtained from the three-dimensional beam geometry and atomic velocity distribution and over the longitudinal velocity distribution. The optical pumping is significant at much lower intensities than saturation and depends strongly on the intensity, beam radius, vapor cell length, and spontaneous-decay branching ratio. The result is in agreement with our earlier steady-state solution for a wide range of parameters and predicts two interesting line-shape features.

AB - We study the influence of optical pumping on Doppler-broadened alkali-metal-atom D line spectra by solving the time-dependent density matrix for an open two-level system. The time-dependent absorption is averaged over the distribution of interaction times obtained from the three-dimensional beam geometry and atomic velocity distribution and over the longitudinal velocity distribution. The optical pumping is significant at much lower intensities than saturation and depends strongly on the intensity, beam radius, vapor cell length, and spontaneous-decay branching ratio. The result is in agreement with our earlier steady-state solution for a wide range of parameters and predicts two interesting line-shape features.

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