New method to generate mid-infrared optical frequency combs for molecular spectroscopy

Dissertation

Research output: ThesisDissertationCollection of Articles

Abstract

In the current study, I experimentally demonstrate a new technique for generating a midinfrared optical frequency comb (OFC). The motivation for this work stems from importance of coherent light sources to molecular spectroscopy, particularly in the mid-infrared region, where the strong fundamental molecular vibration-rotation absorption bands lie. Coherent light sources are needed to provide the best available sensitivity and selectivity in the spectroscopy experiments. As a prelude for the OFC research, an optical parametric oscillator operating close to signal-idler degeneracy was also examined in this thesis.
The OFC generator investigated here is based on cascaded quadratic optical nonlinearities (CQNs), an approach that was first discovered as a part of the current study. By applying the new method inside a continuous-wave pumped optical parametric oscillator (OPO), a highpower mid-infrared OFC was produced by simple near-infrared laser pumping.
Here, I present a rigorous experimental study of the new mid-infrared OFC generator. In particular, I verify the CQN comb mode spacing uniformity and demonstrate tuning of the center wavelength, offset frequency, and the mode spacing of the mid-infrared comb. I also apply a parametric seeding technique to improve the spectral quality of the comb. Furthermore, I demonstrate that the CQN method is capable of generating multioctave-spanning composite frequency combs. These results demonstrate the potential of the new OFC generation method for demanding molecular spectroscopy experiments.
Utilization of an OFC source in field applications of molecular spectroscopy requires a robust and compact experimental platform. At the end of this thesis, I present preliminary results of our work towards miniaturization of the CQN comb generator using an optical waveguide device.
Original languageEnglish
QualificationDoctor Degree
Awarding Institution
  • University of Helsinki
Supervisors/Advisors
  • Halonen, Lauri, Supervisor, External person
  • Vainio, Markku, Supervisor, External person
Award date12 Jun 2018
Publisher
Print ISBNs978-951-51-4313-6
Electronic ISBNs978-951-51-4314-3
Publication statusPublished - 12 Jun 2018
MoE publication typeG5 Doctoral dissertation (article)

Fingerprint

molecular spectroscopy
nonlinearity
generators
theses
coherent light
parametric amplifiers
light sources
spacing
laser pumping
miniaturization
inoculation
stems
optical waveguides
infrared lasers
continuous radiation
platforms
selectivity
tuning
absorption spectra
vibration

Cite this

@phdthesis{69f16c96ea344cb1aca14bc663f52d8a,
title = "New method to generate mid-infrared optical frequency combs for molecular spectroscopy: Dissertation",
abstract = "In the current study, I experimentally demonstrate a new technique for generating a midinfrared optical frequency comb (OFC). The motivation for this work stems from importance of coherent light sources to molecular spectroscopy, particularly in the mid-infrared region, where the strong fundamental molecular vibration-rotation absorption bands lie. Coherent light sources are needed to provide the best available sensitivity and selectivity in the spectroscopy experiments. As a prelude for the OFC research, an optical parametric oscillator operating close to signal-idler degeneracy was also examined in this thesis.The OFC generator investigated here is based on cascaded quadratic optical nonlinearities (CQNs), an approach that was first discovered as a part of the current study. By applying the new method inside a continuous-wave pumped optical parametric oscillator (OPO), a highpower mid-infrared OFC was produced by simple near-infrared laser pumping.Here, I present a rigorous experimental study of the new mid-infrared OFC generator. In particular, I verify the CQN comb mode spacing uniformity and demonstrate tuning of the center wavelength, offset frequency, and the mode spacing of the mid-infrared comb. I also apply a parametric seeding technique to improve the spectral quality of the comb. Furthermore, I demonstrate that the CQN method is capable of generating multioctave-spanning composite frequency combs. These results demonstrate the potential of the new OFC generation method for demanding molecular spectroscopy experiments.Utilization of an OFC source in field applications of molecular spectroscopy requires a robust and compact experimental platform. At the end of this thesis, I present preliminary results of our work towards miniaturization of the CQN comb generator using an optical waveguide device.",
author = "Ville Ulvila",
year = "2018",
month = "6",
day = "12",
language = "English",
isbn = "978-951-51-4313-6",
publisher = "University of Helsinki",
address = "Finland",
school = "University of Helsinki",

}

New method to generate mid-infrared optical frequency combs for molecular spectroscopy : Dissertation. / Ulvila, Ville.

University of Helsinki, 2018. 45 p.

Research output: ThesisDissertationCollection of Articles

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AB - In the current study, I experimentally demonstrate a new technique for generating a midinfrared optical frequency comb (OFC). The motivation for this work stems from importance of coherent light sources to molecular spectroscopy, particularly in the mid-infrared region, where the strong fundamental molecular vibration-rotation absorption bands lie. Coherent light sources are needed to provide the best available sensitivity and selectivity in the spectroscopy experiments. As a prelude for the OFC research, an optical parametric oscillator operating close to signal-idler degeneracy was also examined in this thesis.The OFC generator investigated here is based on cascaded quadratic optical nonlinearities (CQNs), an approach that was first discovered as a part of the current study. By applying the new method inside a continuous-wave pumped optical parametric oscillator (OPO), a highpower mid-infrared OFC was produced by simple near-infrared laser pumping.Here, I present a rigorous experimental study of the new mid-infrared OFC generator. In particular, I verify the CQN comb mode spacing uniformity and demonstrate tuning of the center wavelength, offset frequency, and the mode spacing of the mid-infrared comb. I also apply a parametric seeding technique to improve the spectral quality of the comb. Furthermore, I demonstrate that the CQN method is capable of generating multioctave-spanning composite frequency combs. These results demonstrate the potential of the new OFC generation method for demanding molecular spectroscopy experiments.Utilization of an OFC source in field applications of molecular spectroscopy requires a robust and compact experimental platform. At the end of this thesis, I present preliminary results of our work towards miniaturization of the CQN comb generator using an optical waveguide device.

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