Optical and chemical characterization of aerosols emitted from coal, heavy and light fuel oil, and small-scale wood combustion

Anna K. Frey (Corresponding Author), Karri Saarnio, Heikki Lamberg, Fanni Mylläri, Panu Karjalainen, Kimmo Teinilä, Samara Carbone, Jarkko Tissari, Ville Niemelä, Anna Häyrinen, Jani Rautiainen, Jorma Kytömäki, Paulo Artaxo, Aki Virkkula, Liisa Pirjola, Topi Rönkkö, Jorma Keskinen, Jorma Jokiniemi, Risto Hillamo

Research output: Contribution to journalArticleScientificpeer-review

10 Citations (Scopus)

Abstract

Particle emissions affect radiative forcing in the atmosphere. Therefore, it is essential to know the physical and chemical characteristics of them. This work studied the chemical, physical, and optical characteristics of particle emissions from small-scale wood combustion, coal combustion of a heating and power plant, as well as heavy and light fuel oil combustion at a district heating station. Fine particle (PM1) emissions were the highest in wood combustion with a high fraction of absorbing material. The emissions were lowest from coal combustion mostly because of efficient cleaning techniques used at the power plant. The chemical composition of aerosols from coal and oil combustion included mostly ions and trace elements with a rather low fraction of absorbing material. The single scattering albedo and aerosol forcing efficiency showed that primary particles emitted from wood combustion and some cases of oil combustion would have a clear climate warming effect even over dark earth surfaces. Instead, coal combustion particle emissions had a cooling effect. Secondary processes in the atmosphere will further change the radiative properties of these emissions but are not considered in this study
Original languageEnglish
Pages (from-to)827-836
JournalEnvironmental Science & Technology
Volume48
Issue number1
DOIs
Publication statusPublished - 2014
MoE publication typeA1 Journal article-refereed

Fingerprint Dive into the research topics of 'Optical and chemical characterization of aerosols emitted from coal, heavy and light fuel oil, and small-scale wood combustion'. Together they form a unique fingerprint.

  • Cite this

    Frey, A. K., Saarnio, K., Lamberg, H., Mylläri, F., Karjalainen, P., Teinilä, K., Carbone, S., Tissari, J., Niemelä, V., Häyrinen, A., Rautiainen, J., Kytömäki, J., Artaxo, P., Virkkula, A., Pirjola, L., Rönkkö, T., Keskinen, J., Jokiniemi, J., & Hillamo, R. (2014). Optical and chemical characterization of aerosols emitted from coal, heavy and light fuel oil, and small-scale wood combustion. Environmental Science & Technology, 48(1), 827-836. https://doi.org/10.1021/es4028698