TY - JOUR
T1 - Physical Characteristics of Particle Emissions from a Medium Speed Ship Engine Fueled with Natural Gas and Low-Sulfur Liquid Fuels
AU - Alanen, Jenni
AU - Isotalo, Mia
AU - Kuittinen, Niina
AU - Simonen, Pauli
AU - Martikainen, Sampsa
AU - Kuuluvainen, Heino
AU - Honkanen, Mari
AU - Lehtoranta, Kati
AU - Nyyssönen, Sami
AU - Vesala, Hannu
AU - Timonen, Hilkka
AU - Aurela, Minna
AU - Keskinen, Jorma
AU - Rönkkö, Topi
N1 - Funding Information:
This research was done in HERE (40330/13), funded by Tekes (Business Finland), AGCO Power Oy, Dekati Oy, Dinex Ecocat Oy, Neste Oyj, Pegasor Oy, and Wärtsilä Oy. This work utilized Tampere Microscopy Center facilities at Tampere University.
Publisher Copyright:
© 2020 American Chemical Society.
Copyright:
Copyright 2020 Elsevier B.V., All rights reserved.
PY - 2020/5/5
Y1 - 2020/5/5
N2 - Particle emissions from marine traffic affect significantly air quality in coastal areas and the climate. The particle emissions were studied from a 1.4 MW marine engine operating on low-sulfur fuels natural gas (NG; dual-fuel with diesel pilot), marine gas oil (MGO) and marine diesel oil (MDO). The emitted particles were characterized with respect to particle number (PN) emission factors, PN size distribution down to nanometer scale (1.2-414 nm), volatility, electric charge, morphology, and elemental composition. The size distribution of fresh exhaust particles was bimodal for all the fuels, the nucleation mode highly dominating the soot mode. Total PN emission factors were 2.7 × 1015-7.1 × 1015 #/kWh, the emission being the lowest with NG and the highest with MDO. Liquid fuel combustion generated 4-12 times higher soot mode particle emissions than the NG combustion, and the harbor-area-typical lower engine load (40%) caused higher total PN emissions than the higher load (85%). Nonvolatile particles consisted of nanosized fuel, and spherical lubricating oil core mode particles contained, e.g., calcium as well as agglomerated soot mode particles. Our results indicate the PN emissions from marine engines may remain relatively high regardless of fuel sulfur limits, mostly due to the nanosized particle emissions.
AB - Particle emissions from marine traffic affect significantly air quality in coastal areas and the climate. The particle emissions were studied from a 1.4 MW marine engine operating on low-sulfur fuels natural gas (NG; dual-fuel with diesel pilot), marine gas oil (MGO) and marine diesel oil (MDO). The emitted particles were characterized with respect to particle number (PN) emission factors, PN size distribution down to nanometer scale (1.2-414 nm), volatility, electric charge, morphology, and elemental composition. The size distribution of fresh exhaust particles was bimodal for all the fuels, the nucleation mode highly dominating the soot mode. Total PN emission factors were 2.7 × 1015-7.1 × 1015 #/kWh, the emission being the lowest with NG and the highest with MDO. Liquid fuel combustion generated 4-12 times higher soot mode particle emissions than the NG combustion, and the harbor-area-typical lower engine load (40%) caused higher total PN emissions than the higher load (85%). Nonvolatile particles consisted of nanosized fuel, and spherical lubricating oil core mode particles contained, e.g., calcium as well as agglomerated soot mode particles. Our results indicate the PN emissions from marine engines may remain relatively high regardless of fuel sulfur limits, mostly due to the nanosized particle emissions.
UR - http://www.scopus.com/inward/record.url?scp=85084272900&partnerID=8YFLogxK
U2 - 10.1021/acs.est.9b06460
DO - 10.1021/acs.est.9b06460
M3 - Article
C2 - 32250108
AN - SCOPUS:85084272900
SN - 0013-936X
VL - 54
SP - 5376
EP - 5384
JO - Environmental Science & Technology
JF - Environmental Science & Technology
IS - 9
ER -