Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept

Francisco Vidal Vázquez; Joonas Koponen; Vesa Ruuskanen; Cyril Bajamundi; Antti Kosonen; Pekka Simell; Jero Ahola; Christian Frilund; Jere Elfving; Matti Reinikainen; Niko Heikkinen; Juho Kauppinen; Paolo Piermartini

doi:10.1016/j.jcou.2018.09.026

Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept

Francisco Vidal Vázquez, Joonas Koponen^* (Corresponding Author), Vesa Ruuskanen, Cyril Bajamundi, Antti Kosonen, Pekka Simell, Jero Ahola, Christian Frilund, Jere Elfving, Matti Reinikainen, Niko Heikkinen, Juho Kauppinen, Paolo Piermartini

^*Corresponding author for this work

Research output: Contribution to journal › Article › Scientific › peer-review

111 Citations (Scopus)

Abstract

This work demonstrates hydrocarbon production directly from water, solar energy, and air - called SOLETAIR. The plant includes direct air capture (DAC) of carbon dioxide, hydrogen production by water electrolysis, and two-step synthesis bench-scale units that operate using grid-connected solar photovoltaic (PV) electricity. In addition, co-feeding of hydrogen and carbon monoxide from gas bundles are utilized to enable scaling between units. This pilot plant achieved a total operating time of approx. 300 h with a combined production of oil and wax of 6.2 kg per day. The mass and energy balances in integration of the units are studied. According to the experiments and studies, potential and bottlenecks to improve the individual units and their integration are found. Finally, a conceptual Power-to-X plant is presented, which can achieve energy and carbon efficiencies of 47% and 94%, respectively, considering liquid and solid hydrocarbons as products.

Original language	English
Pages (from-to)	235-246
Number of pages	12
Journal	Journal of CO2 Utilization
Volume	28
Early online date	15 Oct 2018
DOIs	https://doi.org/10.1016/j.jcou.2018.09.026
Publication status	Published - 2018
MoE publication type	A1 Journal article-refereed

Keywords

Carbon capture and utilization
Direct air capture
Fischer-Tropsch synthesis
Power-to-X
Water electrolysis

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1016/j.jcou.2018.09.026

Cite this

Vázquez, F. V., Koponen, J., Ruuskanen, V., Bajamundi, C., Kosonen, A., Simell, P., Ahola, J., Frilund, C., Elfving, J., Reinikainen, M., Heikkinen, N., Kauppinen, J., & Piermartini, P. (2018). Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept. Journal of CO2 Utilization, 28, 235-246. https://doi.org/10.1016/j.jcou.2018.09.026

@article{d46ebf6c4bed4cc298a5ebf84d2fe500,

title = "Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept",

abstract = "This work demonstrates hydrocarbon production directly from water, solar energy, and air - called SOLETAIR. The plant includes direct air capture (DAC) of carbon dioxide, hydrogen production by water electrolysis, and two-step synthesis bench-scale units that operate using grid-connected solar photovoltaic (PV) electricity. In addition, co-feeding of hydrogen and carbon monoxide from gas bundles are utilized to enable scaling between units. This pilot plant achieved a total operating time of approx. 300 h with a combined production of oil and wax of 6.2 kg per day. The mass and energy balances in integration of the units are studied. According to the experiments and studies, potential and bottlenecks to improve the individual units and their integration are found. Finally, a conceptual Power-to-X plant is presented, which can achieve energy and carbon efficiencies of 47% and 94%, respectively, considering liquid and solid hydrocarbons as products.",

keywords = "Carbon capture and utilization, Direct air capture, Fischer-Tropsch synthesis, Power-to-X, Water electrolysis",

author = "V{\'a}zquez, {Francisco Vidal} and Joonas Koponen and Vesa Ruuskanen and Cyril Bajamundi and Antti Kosonen and Pekka Simell and Jero Ahola and Christian Frilund and Jere Elfving and Matti Reinikainen and Niko Heikkinen and Juho Kauppinen and Paolo Piermartini",

note = "Funding Information: TEKES is acknowledged for the main financial support of the SOLETAIR project (soletair.fi). The project partners are also thanked for their financial and in-kind contributions. The SOLETAIR project concept was developed from the work carried out in the Neo-Carbon Energy project (neocarbonenergy.fi). Publisher Copyright: {\textcopyright} 2018 Elsevier Ltd. All rights reserved. Copyright: Copyright 2018 Elsevier B.V., All rights reserved.",

year = "2018",

doi = "10.1016/j.jcou.2018.09.026",

language = "English",

volume = "28",

pages = "235--246",

journal = "Journal of CO2 Utilization",

issn = "2212-9820",

publisher = "Elsevier B.V.",

}

Vázquez, FV, Koponen, J, Ruuskanen, V, Bajamundi, C, Kosonen, A, Simell, P, Ahola, J, Frilund, C , Elfving, J , Reinikainen, M , Heikkinen, N , Kauppinen, J & Piermartini, P 2018, 'Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept', Journal of CO2 Utilization, vol. 28, pp. 235-246. https://doi.org/10.1016/j.jcou.2018.09.026

Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept. / Vázquez, Francisco Vidal; Koponen, Joonas (Corresponding Author); Ruuskanen, Vesa et al.
In: Journal of CO2 Utilization, Vol. 28, 2018, p. 235-246.

Research output: Contribution to journal › Article › Scientific › peer-review

TY - JOUR

T1 - Power-to-X technology using renewable electricity and carbon dioxide from ambient air

T2 - SOLETAIR proof-of-concept and improved process concept

AU - Vázquez, Francisco Vidal

AU - Koponen, Joonas

AU - Ruuskanen, Vesa

AU - Bajamundi, Cyril

AU - Kosonen, Antti

AU - Simell, Pekka

AU - Ahola, Jero

AU - Frilund, Christian

AU - Elfving, Jere

AU - Reinikainen, Matti

AU - Heikkinen, Niko

AU - Kauppinen, Juho

AU - Piermartini, Paolo

N1 - Funding Information: TEKES is acknowledged for the main financial support of the SOLETAIR project (soletair.fi). The project partners are also thanked for their financial and in-kind contributions. The SOLETAIR project concept was developed from the work carried out in the Neo-Carbon Energy project (neocarbonenergy.fi). Publisher Copyright: © 2018 Elsevier Ltd. All rights reserved. Copyright: Copyright 2018 Elsevier B.V., All rights reserved.

PY - 2018

Y1 - 2018

N2 - This work demonstrates hydrocarbon production directly from water, solar energy, and air - called SOLETAIR. The plant includes direct air capture (DAC) of carbon dioxide, hydrogen production by water electrolysis, and two-step synthesis bench-scale units that operate using grid-connected solar photovoltaic (PV) electricity. In addition, co-feeding of hydrogen and carbon monoxide from gas bundles are utilized to enable scaling between units. This pilot plant achieved a total operating time of approx. 300 h with a combined production of oil and wax of 6.2 kg per day. The mass and energy balances in integration of the units are studied. According to the experiments and studies, potential and bottlenecks to improve the individual units and their integration are found. Finally, a conceptual Power-to-X plant is presented, which can achieve energy and carbon efficiencies of 47% and 94%, respectively, considering liquid and solid hydrocarbons as products.

AB - This work demonstrates hydrocarbon production directly from water, solar energy, and air - called SOLETAIR. The plant includes direct air capture (DAC) of carbon dioxide, hydrogen production by water electrolysis, and two-step synthesis bench-scale units that operate using grid-connected solar photovoltaic (PV) electricity. In addition, co-feeding of hydrogen and carbon monoxide from gas bundles are utilized to enable scaling between units. This pilot plant achieved a total operating time of approx. 300 h with a combined production of oil and wax of 6.2 kg per day. The mass and energy balances in integration of the units are studied. According to the experiments and studies, potential and bottlenecks to improve the individual units and their integration are found. Finally, a conceptual Power-to-X plant is presented, which can achieve energy and carbon efficiencies of 47% and 94%, respectively, considering liquid and solid hydrocarbons as products.

KW - Carbon capture and utilization

KW - Direct air capture

KW - Fischer-Tropsch synthesis

KW - Power-to-X

KW - Water electrolysis

UR - http://www.scopus.com/inward/record.url?scp=85054964012&partnerID=8YFLogxK

U2 - 10.1016/j.jcou.2018.09.026

DO - 10.1016/j.jcou.2018.09.026

M3 - Article

AN - SCOPUS:85054964012

SN - 2212-9820

VL - 28

SP - 235

EP - 246

JO - Journal of CO2 Utilization

JF - Journal of CO2 Utilization

ER -

Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept

Abstract

Keywords

UN SDGs

Access to Document

Other files and links

Fingerprint

SOLETAIR: Piloting Research of Renewable Energy System

Cite this

Power-to-X technology using renewable electricity and carbon dioxide from ambient air: SOLETAIR proof-of-concept and improved process concept

Abstract

Keywords

UN SDGs

Access to Document

Other files and links

Fingerprint

Projects

SOLETAIR: Piloting Research of Renewable Energy System

Cite this