Precision spectroscopy of acetylene transitions using an optical frequency synthesizer

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An optical frequency synthesizer is used for saturation spectroscopy of acetylene near 1540 nm. In the synthesizer, a user-specified frequency is generated from an atomic time base by phase locking the second harmonic of a cw near-IR external-cavity diode laser (ECDL) to a Ti:sapphire frequency comb. By stepping the repetition rate of the frequency comb, the ECDL frequency is swept over an acetylene transition in a saturated absorption spectroscopy setup. Hence, a spectral lineshape is measured with an absolute frequency scale. Line-center frequencies determined by fitting theoretical line profiles to the measured data are in good agreement with values measured with the ECDL stabilized to acetylene by third-harmonic locking and with the values recommended by the International Committee for Weights and Measures (CIPM).
Original languageEnglish
Pages (from-to)2619-2621
Number of pages3
JournalOptics Letters
Issue number17
Publication statusPublished - 2009
MoE publication typeA1 Journal article-refereed

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