Reduced anthropogenic aerosol radiative forcing caused by biogenic new particle formation

Hamish Gordon, Kamalika Sengupta, Alexandru Rap, Jonathan Duplissy, Carla Frege, Christina Williamson, Martin Heinritzi, Mario Simon, Chao Yan, João Almeida, Jasmin Tröstl, Tuomo Nieminen, Ismael K. Ortega, Robert Wagner, Eimear M. Dunne, Alexey Adamov, Antonio Amorim, Anne Kathrin Bernhammer, Federico Bianchi, Martin BreitenlechnerSophia Brilke, Xuemeng Chen, Jill S. Craven, Antonio Dias, Sebastian Ehrhart, Lukas Fischer, Richard C. Flagan, Alessandro Franchin, Claudia Fuchs, Roberto Guida, Jani Hakala, Christopher R. Hoyle, Tuija Jokinen, Heikki Junninen, Juha Kangasluoma, Jaeseok Kim, Jasper Kirkby, Manuel Krapf, Andreas Kürten, Ari Laaksonen, Katrianne Lehtipalo, Vladimir Makhmutov, Serge Mathot, Ugo Molteni, Sarah A. Monks, Antti Onnela, Otso Peräkylä, Felix Piel, Tuukka Petäjä, Arnaud P. Praplan, Kirsty J. Pringle, Nigel A.D. Richards, Matti P. Rissanen, Linda Rondo, Nina Sarnela, Siegfried Schobesberger, Catherine E. Scott, John H. Seinfeld, Sangeeta Sharma, Mikko Sipilä, Gerhard Steiner, Yuri Stozhkov, Frank Stratmann, Antonio Tomé, Annele Virtanen, Alexander Lucas Vogel, Andrea C. Wagner, Paul E. Wagner, Ernest Weingartner, Daniela Wimmer, Paul M. Winkler, Penglin Ye, Xuan Zhang, Armin Hansel, Josef Dommen, Neil M. Donahue, Douglas R. Worsnop, Urs Baltensperger, Markku Kulmala, Joachim Curtius, Kenneth S. Carslaw

Research output: Contribution to journalArticleScientificpeer-review

99 Citations (Scopus)

Abstract

The magnitude of aerosol radiative forcing caused by anthropogenic emissions depends on the baseline state of the atmosphere under pristine preindustrial conditions. Measurements show that particle formation in atmospheric conditions can occur solely from biogenic vapors. Here, we evaluate the potential effect of this source of particles on preindustrial cloud condensation nuclei (CCN) concentrations and aerosol-cloud radiative forcing over the industrial period. Model simulations show that the pure biogenic particle formation mechanism has a much larger relative effect on CCN concentrations in the preindustrial atmosphere than in the present atmosphere because of the lower aerosol concentrations. Consequently, preindustrial cloud albedo is increased more than under present day conditions, and therefore the cooling forcing of anthropogenic aerosols is reduced. The mechanism increases CCN concentrations by 20-100% over a large fraction of the preindustrial lower atmosphere, and the magnitude of annual global mean radiative forcing caused by changes of cloud albedo since 1750 is reduced by 0.22 W m-2 (27%) to -0.60 W m-2. Model uncertainties, relatively slow formation rates, and limited available ambient measurements make it difficult to establish the significance of a mechanism that has its dominant effect under preindustrial conditions. Our simulations predict more particle formation in the Amazon than is observed. However, the first observation of pure organic nucleation has now been reported for the free troposphere. Given the potentially significant effect on anthropogenic forcing, effort should be made to better understand such naturally driven aerosol processes.

Original languageEnglish
Pages (from-to)12053-12058
Number of pages6
JournalProceedings of the National Academy of Sciences of the United States of America
Volume113
Issue number43
DOIs
Publication statusPublished - 25 Oct 2016
MoE publication typeA1 Journal article-refereed

Keywords

  • Aerosol
  • Biogenic
  • Climate
  • Forcing

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