Surface tension of a liquid metal-oxygen system using a multilayer free energy model

Risto Pajarre (Corresponding Author), Pertti Koukkari, T. Tanaka

Research output: Contribution to journalArticleScientificpeer-review

3 Citations (Scopus)

Abstract

A constrained free energy model for an interfacial system of interacting layers is derived in the regular solution and Redlich-Kister formalisms. Composition and interfacial energies are solved using a model based on the minimisation of the total free energy of the system with a fixed interfacial area. As example cases iron-oxygen and copper-oxygen surfaces and liquid-liquid metal alloy interfaces are studied.
Original languageEnglish
Pages (from-to)736-747
Number of pages11
JournalInternational Journal of Materials Research
Volume104
Issue number8
DOIs
Publication statusPublished - 2013
MoE publication typeA1 Journal article-refereed

Fingerprint

oxygen supply equipment
liquid metals
Liquid metals
Free energy
Surface tension
interfacial tension
Multilayers
free energy
Oxygen
interfacial energy
oxygen
Interfacial energy
Copper
Iron
iron
copper
optimization
Liquids
liquids
Chemical analysis

Keywords

  • constrained free energy
  • interfacial tension
  • metal-oxygen adsorption
  • surface tension

Cite this

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title = "Surface tension of a liquid metal-oxygen system using a multilayer free energy model",
abstract = "A constrained free energy model for an interfacial system of interacting layers is derived in the regular solution and Redlich-Kister formalisms. Composition and interfacial energies are solved using a model based on the minimisation of the total free energy of the system with a fixed interfacial area. As example cases iron-oxygen and copper-oxygen surfaces and liquid-liquid metal alloy interfaces are studied.",
keywords = "constrained free energy, interfacial tension, metal-oxygen adsorption, surface tension",
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Surface tension of a liquid metal-oxygen system using a multilayer free energy model. / Pajarre, Risto (Corresponding Author); Koukkari, Pertti; Tanaka, T.

In: International Journal of Materials Research, Vol. 104, No. 8, 2013, p. 736-747.

Research output: Contribution to journalArticleScientificpeer-review

TY - JOUR

T1 - Surface tension of a liquid metal-oxygen system using a multilayer free energy model

AU - Pajarre, Risto

AU - Koukkari, Pertti

AU - Tanaka, T.

PY - 2013

Y1 - 2013

N2 - A constrained free energy model for an interfacial system of interacting layers is derived in the regular solution and Redlich-Kister formalisms. Composition and interfacial energies are solved using a model based on the minimisation of the total free energy of the system with a fixed interfacial area. As example cases iron-oxygen and copper-oxygen surfaces and liquid-liquid metal alloy interfaces are studied.

AB - A constrained free energy model for an interfacial system of interacting layers is derived in the regular solution and Redlich-Kister formalisms. Composition and interfacial energies are solved using a model based on the minimisation of the total free energy of the system with a fixed interfacial area. As example cases iron-oxygen and copper-oxygen surfaces and liquid-liquid metal alloy interfaces are studied.

KW - constrained free energy

KW - interfacial tension

KW - metal-oxygen adsorption

KW - surface tension

U2 - 10.3139/146.110921

DO - 10.3139/146.110921

M3 - Article

VL - 104

SP - 736

EP - 747

JO - International Journal of Materials Research

JF - International Journal of Materials Research

SN - 1862-5282

IS - 8

ER -