The influence of carbon impurities on the formation of loops in tungsten irradiated with self-ions

Jari Likonen, Nicolas Castin (Corresponding Author), A Dubinko, G Bonny, Andree De Backer, Andrea Sand, Kalle Heinola, D. Terentyev

Research output: Contribution to journalArticleScientificpeer-review

Abstract

The microstructure changes taking place in W under irradiation are governed by many factors, amongst which C impurities and their interactions with self-interstitial atoms (SIA). In this work, we specifically study this effect by conducting a dedicated 2-MeV self-ions irradiation experiment, at room temperature. Samples were irradiated up to 0.02, 0.15 and 1.2 dpa. Transmission electron microscopy (TEM) expectedly revealed a large density of SIA loops at all these doses. Surprisingly, however, the loop number density increased in a non-monotonous manner with the received dose. Performing chemical analysis with secondary ion spectroscopy measurements (SIMS), we find that our samples were likely contaminated by C injection during the irradiation. Employing an object kinetic Monte Carlo (OKMC) model for microstructure evolution, we demonstrate that the C injection is the likely factor explaining the evolution of loops number density. Our findings highlight the importance of the well-known issue of C injection during ion irradiation experiments, and demonstrate how OKMC models can help to rationalize this effect.
Original languageEnglish
Article number151808
Number of pages8
JournalJournal of Nuclear Materials
Volume527
DOIs
Publication statusPublished - 2019
MoE publication typeA1 Journal article-refereed

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Tungsten
Ion bombardment
tungsten
Carbon
Irradiation
Impurities
Ions
injection
ion irradiation
impurities
Atoms
Microstructure
Kinetics
carbon
interstitials
dosage
microstructure
ions
irradiation
Experiments

Cite this

Likonen, Jari ; Castin, Nicolas ; Dubinko, A ; Bonny, G ; De Backer, Andree ; Sand, Andrea ; Heinola, Kalle ; Terentyev, D. / The influence of carbon impurities on the formation of loops in tungsten irradiated with self-ions. In: Journal of Nuclear Materials. 2019 ; Vol. 527.
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abstract = "The microstructure changes taking place in W under irradiation are governed by many factors, amongst which C impurities and their interactions with self-interstitial atoms (SIA). In this work, we specifically study this effect by conducting a dedicated 2-MeV self-ions irradiation experiment, at room temperature. Samples were irradiated up to 0.02, 0.15 and 1.2 dpa. Transmission electron microscopy (TEM) expectedly revealed a large density of SIA loops at all these doses. Surprisingly, however, the loop number density increased in a non-monotonous manner with the received dose. Performing chemical analysis with secondary ion spectroscopy measurements (SIMS), we find that our samples were likely contaminated by C injection during the irradiation. Employing an object kinetic Monte Carlo (OKMC) model for microstructure evolution, we demonstrate that the C injection is the likely factor explaining the evolution of loops number density. Our findings highlight the importance of the well-known issue of C injection during ion irradiation experiments, and demonstrate how OKMC models can help to rationalize this effect.",
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The influence of carbon impurities on the formation of loops in tungsten irradiated with self-ions. / Likonen, Jari; Castin, Nicolas (Corresponding Author); Dubinko, A; Bonny, G; De Backer, Andree; Sand, Andrea; Heinola, Kalle; Terentyev, D.

In: Journal of Nuclear Materials, Vol. 527, 151808, 2019.

Research output: Contribution to journalArticleScientificpeer-review

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T1 - The influence of carbon impurities on the formation of loops in tungsten irradiated with self-ions

AU - Likonen, Jari

AU - Castin, Nicolas

AU - Dubinko, A

AU - Bonny, G

AU - De Backer, Andree

AU - Sand, Andrea

AU - Heinola, Kalle

AU - Terentyev, D.

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