Abstract
Controlling thermal energy transfer at the nanoscale and thermal properties has become critically important in many applications since it often limits device performance. In this study, the effects on thermal conductivity arising from the nanoscale structure of free-standing nanocrystalline silicon films and the increasing surface-to-volume ratio when fabricated into suspended optomechanical nanobeams are studied. Thermal transport and elucidate the relative impact of different grain size distributions and geometrical dimensions on thermal conductivity are characterized. A micro time-domain thermoreflectance method to study free-standing nanocrystalline silicon films and find a drastic reduction in the thermal conductivity, down to values below 10 W m–1 K–1 is used, with a stronger decrease for smaller grains. In optomechanical nanostructures, this effect is smaller than in membranes due to the competition of surface scattering in decreasing thermal conductivity. Finally, a novel versatile contactless characterization technique that can be adapted to any structure supporting a thermally shifted optical resonance is introduced. The thermal conductivity data agrees quantitatively with the thermoreflectance measurements. This study opens the way to a more generalized thermal characterization of optomechanical cavities and to create hot-spots with engineered shapes at the desired position in the structures as a means to study thermal transport in coupled photon-phonon structures.
| Original language | English |
|---|---|
| Article number | 2105767 |
| Number of pages | 10 |
| Journal | Advanced Functional Materials |
| Volume | 32 |
| Issue number | 4 |
| Early online date | 23 Oct 2021 |
| DOIs | |
| Publication status | Published - 19 Jan 2022 |
| MoE publication type | A1 Journal article-refereed |
Funding
This work was supported by the European Commission FET Open project PHENOMEN (G.A. Nr. 713450). ICN2 was supported by the S. Ochoa program from the Spanish Research Agency (AEI, grant no. SEV‐2017‐0706) and by the CERCA Programme / Generalitat de Catalunya. ICN2 authors acknowledge the support from the Spanish MICINN project SIP (PGC2018‐101743‐B‐I00). D.N.U. and M.F.C. acknowledge the support of a Ramón y Cajal postdoctoral fellowship (RYC‐2014‐15392) and a Severo Ochoa studentship, respectively. E.C.A. acknowledges financial support from the EU FET Open Project NANOPOLY. (GA 829061). A.M. acknowledges support from Ministerio de Ciencia, Innovación y Universidades (grant PGC2018‐094490‐B, PRX18/00126) and Generalitat Valenciana (grants PROMETEO/2019/123, and IDIFEDER/2018/033).
Keywords
- nanostructured materials
- optomechanics
- phonons
- polycrystalline
- silicon
- thermal characterization methods
- thermal conduction
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