Versatile high energy X-ray transparent electrolysis cell for operando measurements

Asger B.  Moss; Joel Hätinen; Peter Kúš; Sahil Garg; Marta Mirolo; Ib Chorkendorff; Brian Seger; Jakub Drnec

doi:10.1016/j.jpowsour.2023.232754

Versatile high energy X-ray transparent electrolysis cell for operando measurements

Asger B. Moss, Joel Hätinen, Peter Kúš, Sahil Garg, Marta Mirolo, Ib Chorkendorff, Brian Seger, Jakub Drnec^*

^*Corresponding author for this work

Not published at VTT

Research output: Contribution to journal › Article › Scientific › peer-review

18 Citations (Scopus)

Abstract

Herein we present a design for a versatile electrochemical cell for High Energy X-ray operando studies of Membrane Electrode Assembly (MEA) based electrochemical systems. The cell flowplate materials can be interchanged according to the needs of experiments, allowing studies of different chemistries and reactions. The design also allows for coupling the X-ray elastic scattering techniques with computed tomography reconstruction, opening the possibility of 3D mapping of chemical and structural properties in operating devices. The cell has originally been designed and tested for CO2 electrolysis performance studies using Wide Angle X-ray Scattering (WAXS) technique.

Original language	English
Article number	232754
Journal	Journal of Power Sources
Volume	562
DOIs	https://doi.org/10.1016/j.jpowsour.2023.232754
Publication status	Published - 1 Apr 2023
MoE publication type	A1 Journal article-refereed

Funding

AM, SG, IC, BS would like to acknowledge the funding from Villum Fonden, part of the Villum Center for the Science of Sustainable Fuels and Chemicals (V-SUSTAIN grant 9455, E-Tunneling grant 36254), as well as the ECOEthylene project from Innovation Fund Denmark (Grant# 8057-00018B). PK would like to acknowledge project Mobility 8J21FR019 from MSMT Czech Republic for funding. JD and PK would like to acknowledge Campus France (grant PHC Barrande 46755RA) for funding. We acknowledge the European Synchrotron Radiation Facility (ESRF) for the provision of synchrotron radiation using beamline ID 31. AM, SG, IC, BS would like to acknowledge the funding from Villum Fonden , part of the Villum Center for the Science of Sustainable Fuels and Chemicals (V-SUSTAIN grant 9455 , E-Tunneling grant 36254 ), as well as the ECOEthylene project from Innovation Fund Denmark (Grant# 8057-00018B ). PK would like to acknowledge project Mobility 8J21FR019 from MSMT Czech Republic for funding. JD and PK would like to acknowledge Campus France (grant PHC Barrande 46755RA ) for funding. We acknowledge the European Synchrotron Radiation Facility (ESRF) for the provision of synchrotron radiation using beamline ID 31.

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1016/j.jpowsour.2023.232754

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title = "Versatile high energy X-ray transparent electrolysis cell for operando measurements",

abstract = "Herein we present a design for a versatile electrochemical cell for High Energy X-ray operando studies of Membrane Electrode Assembly (MEA) based electrochemical systems. The cell flowplate materials can be interchanged according to the needs of experiments, allowing studies of different chemistries and reactions. The design also allows for coupling the X-ray elastic scattering techniques with computed tomography reconstruction, opening the possibility of 3D mapping of chemical and structural properties in operating devices. The cell has originally been designed and tested for CO2 electrolysis performance studies using Wide Angle X-ray Scattering (WAXS) technique.",

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doi = "10.1016/j.jpowsour.2023.232754",

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T1 - Versatile high energy X-ray transparent electrolysis cell for operando measurements

AU - Moss, Asger B.

AU - Hätinen, Joel

AU - Kúš, Peter

AU - Garg, Sahil

AU - Mirolo, Marta

AU - Chorkendorff, Ib

AU - Seger, Brian

AU - Drnec, Jakub

PY - 2023/4/1

Y1 - 2023/4/1

N2 - Herein we present a design for a versatile electrochemical cell for High Energy X-ray operando studies of Membrane Electrode Assembly (MEA) based electrochemical systems. The cell flowplate materials can be interchanged according to the needs of experiments, allowing studies of different chemistries and reactions. The design also allows for coupling the X-ray elastic scattering techniques with computed tomography reconstruction, opening the possibility of 3D mapping of chemical and structural properties in operating devices. The cell has originally been designed and tested for CO2 electrolysis performance studies using Wide Angle X-ray Scattering (WAXS) technique.

AB - Herein we present a design for a versatile electrochemical cell for High Energy X-ray operando studies of Membrane Electrode Assembly (MEA) based electrochemical systems. The cell flowplate materials can be interchanged according to the needs of experiments, allowing studies of different chemistries and reactions. The design also allows for coupling the X-ray elastic scattering techniques with computed tomography reconstruction, opening the possibility of 3D mapping of chemical and structural properties in operating devices. The cell has originally been designed and tested for CO2 electrolysis performance studies using Wide Angle X-ray Scattering (WAXS) technique.

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DO - 10.1016/j.jpowsour.2023.232754

M3 - Article

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VL - 562

JO - Journal of Power Sources

JF - Journal of Power Sources

M1 - 232754

ER -

Versatile high energy X-ray transparent electrolysis cell for operando measurements

Abstract

Funding

UN SDGs

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